赵英博

赵英博课题组介绍

课题组长丨研究介绍丨发表论文丨本组成员

课题组长

赵英博，助理教授、研究员、独立课题组长

电子邮件：zhaoyb2@xdjzhibo.com

实验室：小妲己直播 2号楼509

教育及研究经历

2008-2012, 中国科学技术大学少年班小妲己直播，化学专业，学士学位

2012-2017, 加州大学伯克利分校化学系，博士学位 (导师：Omar Yaghi 院士）

2017-2021, 加州大学伯克利分校电子工程系，博士后研究员(合作导师：Ali Javey教授）

2021年8月- 小妲己直播助理教授，研究员

研究介绍

研究方向

课题组研究方向包括框架材料的合成、物性研究及其器件应用。主要研究的材料体系是MOF玻璃和新概念COF，主要发展的应用是离子传导和光电器件。

【20240516 -小妲己直播赵英博-框架材料的发展历史与前沿】

//www.bilibili.com/video/BV16x4y1W72V/?share_source=copy_web&vd_source=8c7a6eeb864156b010004c6b74dfa3c5

发表论文

2024

Hsueh, C.-H., He, C., Tan, X., Zhu, H., Cheong, W.-C., Li, A.-Z., Duan, H., Zhao, Y*., Chen, C*.; Three-Dimensional Mesoporous Covalent Organic Framework for Photocatalytic Oxidative Dehydrogenation to Quinoline. J. Am. Chem. Soc. 2024, //doi.org/10.1021/jacs.4c12286

（第一作者清华大学陈晨课题组薛州宏）

Wei, L#., Wu, S#., Li, C., Liu, C., Chen, H., Zhang, Y.-B*., Zheng, F*., Ma, Y*., Zhao, Y*; Dimensionality and Molecular Packing Control of Covalent Organic Frameworks through Pendant Group Design. J. Am. Chem. Soc. 2024, 146, 31384–31390.

（第一作者助理研究员魏蕾，马延航课题组吴诗韬）

Zhang, Z., Zhao, Y*; Transparent and high-porosity aluminum alkoxide network-forming glasses. Nat. Commun 15, 7339.

(第一作者 2021级硕士张紫惠）

Wei, L#., Hai, X#., Xu, T., Wang, Z., Jiang, W., Jiang, S., Wang, Q., Zhang, Y.-B*., Zhao, Y*; Encoding ordered structural complexity to covalent organic frameworks. Nat. Commun. 15, 2411.

（第一作者助理研究员魏蕾，2021级硕士海馨月）

Qi, A., Li, C., Evans, J., Zhao, Y*., Li, Tao*; Self-sorting of Interfacial Compatibility in MOF-based Mixed Matrix Membranes. Angew. Chem. Int. Ed.,e202400474.

（第一作者 2021级李涛组联合培养硕士齐安恒）

Huang, Y., Qi, A., Li, S., Tang, Lu., Zhao, Y*., Li, Tao*; Rapid coating of polyamide, polyurea, and polythiourea on metal–organic framework surfaces. APL Mater. 12, 031116 (2024)

（第一作者 2021级李涛组联合培养硕士黄云梅）

2023

Zhang, Y.,# Liu, Y.,# Bao, W., Zhang, X., Yan, P., Yao, X., Chen, M.-Z., Xie, T-Y., Cao, L., Cai, X., Li, H., Deng, Y., Zhao, L., Zeng, M-H., Jiang, S., Zhao, Y.,^*Xie, J.^*; Monolithic Titanium Alkoxide Networks for Lithium-Ion Conductive All-Solid-State Electrolytes. Nano Lett.2023, 23, 4066–4073.

（第一作者谢琎课题组张悦，本课题组 2021级硕士刘盈）

Chen, M.-Z., Li, J., Liao, S., Guo, Y. -H., Liu, T., Ma, R. -F., Xie, T. -Y., Liu, W. -D., Peng, S. -X., Kuang, X., Yin, Z.,* Zhao, Y.,* Zeng, M.-H.,*; Multi-stage Transformations of a Cluster-Based Metal-Organic Framework: Perturbing Crystals to Glass-Forming Liquids that Re-Crystallize at High Temperature. Angew. Chem. Int. Ed, e202305942.

（第一作者 2021年访问生，广西师范大学曾明华课题组2020级硕士陈明珠）

Yin, Z.,^* Zhao, Y.,^* Zeng, M.-H.,^* Challenge, Advance and Emerging Opportunities for Metal-Organic Framework Glasses: from Dynamic Chemistry to Material Science and Noncrystalline Physics. Acta Chimica Sinica, 2023, 81, 246-252.

Bao, W.; Zhang, Y.; Cao, L.; Jiang, Y.; Zhang, H.; Zhang, N.; Liu, Y.; Yan, P.; Wang, X.; Liu, Y.; Li, H.; Zhao, Y.; Xie, J.*; A H₂O-initiated crosslinking strategy for ultrafine nanoclusters reinforced high toughness polymer-in-plasticizer solid electrolyte Adv. Mater. 2023, 2304712. //doi.org/10.1002/adma.202304712

Xu, Y.; Sun, T.; Zeng, T.; Zhang, X.; Yao, X.; Liu, S.; Shi, Z.; Wen, W.; Zhao, Y.; Jiang, S.; Ma, Y.; Zhang, Y.-B.*; Symmetry-breaking dynamics in a tautomeric 3D covalent organic framework. Nat. Commun. 2023, 14, 4215.

Zhang, X.; Xu, Z.; Wang, Z.; Liu, H.; Zhao, Y.; Jiang, S.*; High-throughput and machine learning approaches for the discovery of metal organic frameworks. APL Materials, 2023, 11, 060901, 8 pp.

Liu, T.; Fu, Q.; Li, Y.; Han, X.; Wang, S.; Taniguchi, T.; Watanabe, K.; Wan, D.; Zhang, Q.; Zhao, Y.; Ni, Z.; Ding, F.; Hu, Z,; Yuan, X.*; Lu, J.*; Silver nanoparticle-induced enhancement of light extraction in two-dimensional light-emitting diodes. Optics Letters, 2023, 48, 4372-5.

2022

Yin, Z.,; Zhao, Y.,; Wan, S.,; Yang, J.,; Shi, Z.,; Peng, S.-X.,; Chen, M.-Z.,; Xie, T.-Y.,; Zeng, T.-W.,; Yamamuro, O.,; Nirei, M.,; Akiba, H.,; Zhang, Y.-B.,^*; Yu, H.-B.,^*; Zeng, M.-H.,^*; Synergistic Stimulation of Metal–Organic Frameworks for Stable Super-cooled Liquid and Quenched Glass, J. Am. Chem. Soc. 2022, 144 (29), 13021-13025.

Wei, L^#., Sun, T^#., Shi, Z. Xu, Z., Wen, W., Jiang, S., Zhao, Y^*., Ma, Y^*., Zhang, Y.-B^*.; Guest-adaptive molecular sensing in a dynamic 3D covalent organic framework. Nat Commun 2022, 13, 7936. //doi.org/10.1038/s41467-022-35674-8

独立工作前主要论文

分子框架材料新结构

Liu, Y^#., Ma, Y^#., Zhao, Y^#., Sun, X., Gándara, F., Furukawa, H., Liu, Z., Zhu, H., Zhu, C., Suenaga, K., Oleynikov, P., Alshammari, A. S., Zhang, X., Terasaki, O.* & Yaghi, O. M.*; Weaving of Organic Threads into a Crystalline Covalent Organic Framework. Science 351, 365-369, (2016).

Science封面论文

Zhao, Y., Lee, S-Y., Becknell, N., Yaghi, O. M.^*, & Angell, C.A.^*; Nanoporous Transparent MOF Glasses with Accessible Internal Surface. J. Am. Chem. Soc.138, 10818-10821, (2016).

Selected as JACS spotlight

Zhao, Y^#., Guo, L^#., Gándara, F., Ma, Y., Liu, Z., Zhu, C., Lyu, H., Trickett, C., Kapustin, E., Terasaki, O., Yaghi, O. M.^*; A Synthetic Route for Crystals of Woven Structures, Monodisperse Nanocrystals, and Thin Films of Covalent Organic Frameworks. J. Am. Chem. Soc. 139, 13166–13172, (2017).

Jiang, J^#., Zhao, Y.^#., & Yaghi, O. M.^*; Covalent Chemistry beyond Molecules. J. Am. Chem. Soc. 138, 3255-3265, (2016).

Selected as JACS spotlight

分子框架的界面控制与功能

Zhao, Y^#., Kornienko, N.^#, Liu, Z., Zhu, C., Asahina, S., Kuo, T.-R., Bao, W., Xie, C., Hexemer, A., Terasaki, O., Yang, P.^* & Yaghi, O. M.^*; Mesoscopic Constructs of Ordered and Oriented Metal-organic Frameworks on Plasmonic Silver Nanocrystals. J. Am. Chem. Soc. 137, 2199-2202, (2015).

Kornienko, N.^#, Zhao, Y.^#, Kley, C. S., Zhu, C., Kim, D., Lin, S., Chang, C. J., Yaghi, O. M.^* & Yang, P.^*; Metal-organic Frameworks for Electrocatalytic Reduction of Carbon Dioxide. J. Am. Chem. Soc. 137, 14129-14135, (2015).

Zhao, H.^#, Zhao, Y.^#, Song, Y., Zhou, M., Lv, W., Tao, L., Feng, Y., Song, B., Ma, Y., Zhang, J., Xiao, J., Wang, Y., Lien, D.-H., Amani, M., Kim, H., Chen, X., Wu, Z., Ni, Z., Wang P., Shi, Y., Ma, H.^*, Zhang, X., Xu, J.-B., Troisi, A., Javey, A.^*, Wang, X.^*; Strong optical response and light emission from a monolayer molecular crystal. Nat. Commun., 10, 1-9, (2019).

Nat. Commun.年度top50物理学论文

Zhao, Y., Wang, V., Javey, A.^*; Molecular materials with short radiative lifetime for high-speed light-emitting devices. Matter, 3, 1832-1844,(2020).

功能器件设计与构筑

Zhao, Y.^#, Wang, V.^#, Lien, D.-H.^#, Javey, A.^*; Generic electroluminescent device for emission from infrared to ultraviolet wavelengths. Nat. Electron.,3, 612–621,(2020).

Wang, V., Zhao, Y., Javey, A.^*; Performance limits of an alternating current electroluminescent device. Adv. Mater., 33, 2005635, (2021).

Nyein, H.Y.Y.^#, Bariya, M.^#, Kivimäki, L., Uusitalo, S., Liaw, T. S., Jansson, E., Ahn, C. H., Hangasky, J.A., Zhao, J., Lin, Y., Happonen, T., Chao, M., Liedert, C., Zhao, Y., Tai, L.-C., Hiltunen, J., Javey, A.^*; Regional and correlative sweat analysis using high-throughput microfluidic sensing patches toward decoding sweat. Sci. Adv., 5, eaaw9906, (2019).

Ji, W., Zhao, Y., Fahad, H.M., Bullock, J., Allen, T., Lien, D.-H., Wolf, S.D., Javey, A.^*; Dip coating passivation of crystalline silicon by lewis acids. ACS nano, 13, 3723-3729, (2019).

Bariya, M.^#, Shahpar, Z.^#, Park, H., Sun, J., Jung, Y., Gao, W., Nyein, H.Y.Y., Liaw, T. S., Tai, L.-C., Ngo, Q. P., Chao, M., Zhao, Y., Hettick, M., Cho, G.^*, Javey, A.^*; Roll-to-Roll gravure printed electrochemical sensors for wearable and medical devices. ACS nano, 12, 6978-6987, (2018).